• 文献标题:   Giant Two-Photon Absorption in Bilayer Graphene
  • 文献类型:   Article
  • 作  者:   YANG HZ, FENG XB, WANG Q, HUANG H, CHEN W, WEE ATS, JI W
  • 作者关键词:   bilayer graphene, twophoton absorption, secondorder perturbation thoery, zscan, ballistic photocurrent
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984
  • 通讯作者地址:   Natl Univ Singapore
  • 被引频次:   114
  • DOI:   10.1021/nl200587h
  • 出版年:   2011

▎ 摘  要

We present a quantum perturbation theory on two-photon absorption (2PA) in monolayer and bilayer graphene which is Bernal-stacked. The theory shows that 2PA is significantly greater in bilayer graphene than monolayer graphene in the visible and infrared spectrum (up to 3 mu m) with a resonant 2PA coefficient of up to similar to 0.2 cm/W located at half of the bandgap energy, gamma(1) = 0.4 eV. In the visible and terahertz region, 2PA exhibits a light frequency dependence of omega(-3) in bilayer graphene, while it is proportional to omega(-4) for monolayer graphene at all photon energies. Within the same order of magnitude, the 2PA theory is in agreement with our Z-scan measurements on high-quality epitaxial bilayer graphene deposited on SiC substrate at light wavelength of 780 and 1100 nm.