• 文献标题:   Rationally designed 1D Ag@AgVO3 nanowire/graphene/protonated g-C3N4 nanosheet heterojunctions for enhanced photocatalysis via electrostatic self-assembly and photochemical reduction methods
  • 文献类型:   Article
  • 作  者:   ZHANG SW, LI JX, WANG XK, HUANG YS, ZENG MY, XU JZ
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS CHEMISTRY A
  • ISSN:   2050-7488 EI 2050-7496
  • 通讯作者地址:   North China Elect Power Univ
  • 被引频次:   146
  • DOI:   10.1039/c5ta00635j
  • 出版年:   2015

▎ 摘  要

1D Ag@AgVO3 nanowire/graphene/protonated g-C3N4 nanosheet (Ag@AgVO3/rGO/PCN) heterojunctions are fabricated via a simple electrostatic self-assembly process followed by a photochemical reduction method. In this hybrid structure, 1D Ag@AgVO3 nanowire spenetrate through 2D nanosheets (graphene and PCN), forming a 3D hybrid photocatalyst, which is applied as an efficient visible light driven photocatalyst for organic pollutant degradation. Its enhanced photocatalytic activity is ascribed to the well-known electronic conductivity of 2D graphene, the intense visible light absorption of 1D Ag@AgVO3 nanowires, large surface areas and rapid photogenerated charge interface transfer and separation. Our results provide a facile way to fabricate hierarchical g-C3N4-based photocatalysts in a controlled manner and highlight promising prospects by adopting an integrative 1D and 2D nanomaterial strategy to design more efficient semiconductor-based composite photocatalysts with high photocatalytic activities and a wide spectral response toward environmental and energy applications.