• 文献标题:   Fabrication, Characterization, and Testing of Graphene Oxide and Hydrophilic Polymer Graphene Oxide Composite Membranes in a Dead-End Flow System
  • 文献类型:   Article
  • 作  者:   MEDINA VF, GRIGGS CS, PETERY B, MATTEISOSA J, GURTOWSKI L, WAISNER SA, BLODGET J, MOSER R
  • 作者关键词:   graphene oxide, membrane treatment, pressure/flux, methylene blue, chitosan, composite
  • 出版物名称:   JOURNAL OF ENVIRONMENTAL ENGINEERING
  • ISSN:   0733-9372 EI 1943-7870
  • 通讯作者地址:   US Army
  • 被引频次:   1
  • DOI:   10.1061/(ASCE)EE.1943-7870.0001268
  • 出版年:   2017

▎ 摘  要

Graphene oxide (GO) has emerged as a promising material for next-generation water treatment membranes. In this study, three types of GO membranes were produced and tested. Both GO and graphene oxide plus polyvinyl alcohol (GO/PVA) membranes were produced using the vacuum-assisted self-assembly (VASA) method, and a chitosan and graphene oxide composite membrane (CSGO) was assembled using GO as a nanoscale filler via evaporation under reduced pressure. Scanning electron micrographs (SEMs) confirmed that GO and GO/ PVA membranes were particularly well ordered, whereas CSGO exhibited reduced ordering attributed to structural and composition differences of GO and CS. The fabricated membranes were tested in a dead-end flow system indicating that each membrane containing GO produced a higher flux at 413 kPa pressure relative to conventional polyamide reverse osmosis (RO) membranes used for benchmark comparison, but was lower in flux to a nanofiltration (NF) membrane. Challenging the membranes with 7.5 mg/L methylene blue solution resulted in >= 97.5% removal of the dye by all three of the membranes. (C) 2017 American Society of Civil Engineers.