• 文献标题:   Facile Approach to Preparation of Nitrogen-doped Graphene and Its Supercapacitive Performance
  • 文献类型:   Article
  • 作  者:   FENG YQ, TANG FL, LANG JW, LIU WW, YAN XB
  • 作者关键词:   graphene, nitrogendoped, solvothermal, supercapacitor
  • 出版物名称:   JOURNAL OF INORGANIC MATERIALS
  • ISSN:   1000-324X
  • 通讯作者地址:   Lanzhou Univ Technol
  • 被引频次:   5
  • DOI:   10.3724/SP.J.1077.2013.12746
  • 出版年:   2013

▎ 摘  要

Nitrogen-doped graphene nanosheets (N-GNSs) with good morphologies were successfully synthesized by a facile solvothermal method. The result of X-ray photoelectron spectroscope (XPS) revealed that most oxygen containing functional groups on the surface of graphene oxide (GO) were removed during solvothermal reduction, and nitrogen atoms from dimethylformamide (DMF) were effectively doped into graphene structure in the form of pyrrolic-N and graphite-N. As an electro-active material, the N-GNSs exhibited superior capacitive behavior in 2 mol/L KOH electrolyte with a high specific capacitance of 181.3 F/g at the current density of 0.5 A/g. Also, it displayed good electrochemical stability with 92.5% of the initial capacitance over consecutive 2000 cycles. Therefore, the N-GNSs can be an attractive candidate as electrode materials for supercapacitors.