▎ 摘　　要

We synthesized the novel nanocomposite consisting alternately of a stacked single graphene sheet and a C-60 monolayer by using the graphite intercalation technique in which alkylamine molecules help intercalate large C-60 molecules into the graphite. Moreover, it is found that the intercalated C-60 molecules can rotate in between single graphene sheets by using C-13 NMR measurements. This preparation method provides a general way for intercalating huge fullerene molecules into graphite, which will lead to promising materials with novel mechanical, physical, and electrical properties.