• 文献标题:   Femtosecond pump-probe spectroscopy of graphene oxide in water
  • 文献类型:   Article
  • 作  者:   SHANG JZ, MA L, LI JW, AI W, YU T, GURZADYAN GG
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF PHYSICS DAPPLIED PHYSICS
  • ISSN:   0022-3727 EI 1361-6463
  • 通讯作者地址:   Nanyang Technol Univ
  • 被引频次:   11
  • DOI:   10.1088/0022-3727/47/9/094008
  • 出版年:   2014

▎ 摘  要

Transient absorption properties of aqueous graphene oxide (GO) have been studied by use of femtosecond pump-probe spectroscopy. Excited state absorption and photobleaching are observed in the wide spectral range. The observed fast three lifetime components are attributed to the absorption of upper excited states and localized states, which is confirmed by both laser induced absorption and transmission kinetics. The longest time component is assigned to the lowest excited state of GO, which mainly originates from the sp2 domains. With the increase of the excitation power, two-quantum absorption occurs, which results in an additional rise-time component of the observed transients.