• 文献标题:   Flexible Salt-Rejecting Photothermal Paper Based on Reduced Graphene Oxide and Hydroxyapatite Nanowires for High-Efficiency Solar Energy-Driven Vapor Generation and Stable Desalination
  • 文献类型:   Article
  • 作  者:   XIONG ZC, ZHU YJ, QIN DD, YANG RL
  • 作者关键词:   hydroxyapatite, nanowire, graphene oxide, salt resistance, seawater desalination
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244 EI 1944-8252
  • 通讯作者地址:   Chinese Acad Sci
  • 被引频次:   1
  • DOI:   10.1021/acsami.0c05986
  • 出版年:   2020

▎ 摘  要

Vapor generation using solar energy is emerging as an efficient technology for wastewater purification and seawater desalination to relieve global water crisis. However, salt deposition on the evaporation surface seriously impairs the long-term steady water evaporation performance. Herein, the flexible salt-rejecting photothermal paper comprising reduced graphene oxide (rGO) and ultralong hydroxyapatite nanowires (HNs) has been developed for high-performance solar energy-driven water evaporation and stable desalination of seawater. The rGO/HN photothermal paper has advantages such as the hierarchical porous structure, interconnected channels, high mechanical strength, high efficiencies of solar light absorption and photothermal conversion, fast water transportation, and good heat insulation and salt-rejecting properties. Furthermore, the hydrophilicity and hydrophobicity of the rGO/HN photothermal paper can be adjusted by regulating the thermal treatment time. The water evaporation rate and energy efficiency of the hydrophilic rGO/HN photothermal paper are 1.48 kg m(-2) h(-1) and 89.2%, respectively, under 1 sun illumination (1 kW m(-2)). The hydrophobic rGO/HN photothermal paper shows a long-time stable water evaporation and salt-rejecting performance in the process of seawater desalination. The flexible salt-rejecting rGO/HN photothermal paper can produce clean water from wastewater and seawater with high rejection rates of organic dyes, metal ions, and salt ions, and it is promising for applications in water purification and seawater desalination.