▎ 摘　　要

Silicone rubber (SR) composites were fabricated using poplar leaves graphene (PG). PG was synthesized from poplar leaves and modified-poplar leaves graphene (MPG) was obtained by treating graphene with a silane coupling agent gamma-aminopropyltriethoxysilane (KH550). The biosynthesized PG and MPG were characterized by using organic elemental analysis, X-ray photoelectron spectroscopy, atomic force microscopy and scanning electron microscopy (SEM). The PG-modified SR composites were studied by using their mechanical properties, Fourier transform infrared spectroscopy, SEM and thermogravimetric analysis. The results showed that the PG synthesized by poplar leaves had high-carbon content and purity. The MPG was more evenly dispersed into SR than the PG, the mechanical properties of the MPG/SR composites were better than those of the PG/SR when the MPG content was 0.1 phr (parts per hundred rubber), the tensile strength and elongation at break were increased by 36.2 and 19.4% respectively and the wear resistance was increased by 57.1%. The thermal stability of the MPG/SR was higher than that of the PG/SR and SR. This important discovery could not only solve the problem of the origin of graphene, but also broaden the application of SR composites.