▎ 摘　　要

Graphene nanowalls (GNWs) were grown directly on carbon fibers using a chemical vapor deposition technique which is simple and catalyst-free. We found that there is very strong pi-pi stacking which is a benefit for the GNWs/carbon fiber interface. This single modified filament then was embedded into an epoxy matrix to be a single-fiber composite in which was formed a "tenonmortise" structure. Such a "tenon-mortise" model provides a simple, stable, and powerful connection between carbon fiber and the epoxy matrix. In addition, it was demonstrated that the epoxy matrix can be well embedded into GNWs through a field emission scanning electron microscope. The results of the single-fiber composite tests indicated that the interfacial strength of the composites was immensely improved by 173% compared to those specimens without GNWs. Published by AIP Publishing.