• 文献标题:   High thermoelectric performance in graphene nanoribbons by graphene/BN interface engineering
  • 文献类型:   Article
  • 作  者:   TRAN VT, SAINTMARTIN J, DOLLFUS P
  • 作者关键词:   graphene ribbon, graphene/bn, seebeck effect, phonon, thermoelectric
  • 出版物名称:   NANOTECHNOLOGY
  • ISSN:   0957-4484 EI 1361-6528
  • 通讯作者地址:   Univ Paris 11
  • 被引频次:   25
  • DOI:   10.1088/0957-4484/26/49/495202
  • 出版年:   2015

▎ 摘  要

The thermoelectric properties of in-plane heterostructures made of Graphene and hexagonal boron nitride (BN) have been investigated by means of atomistic simulation. The heterostructures consist in armchair graphene nanoribbons to the sides of which BN flakes are periodically attached. This arrangement generates a strong mismatch of phonon modes between the different sections of the ribbons, which leads to a very small phonon conductance, while the electron transmission is weakly affected. In combination with the large Seebeck coefficient resulting from the BN-induced bandgap opening or broadening, it is shown that large thermoelectric figure of merit ZT > 0.8 can be reached in perfect structures at relatively low Fermi energy, depending on the graphene nanoribbon width. The high value ZT = 1.48 may even be achieved by introducing appropriately vacancies in the channel, as a consequence of further degradation of the phonon conductance.