• 文献标题:   Preparation and Specific Capacitance Properties of Sulfur, Nitrogen Co-Doped Graphene Quantum Dots
  • 文献类型:   Article
  • 作  者:   OUYANG Z, LEI Y, CHEN YP, ZHANG Z, JIANG ZC, HU JX, LIN YY
  • 作者关键词:   graphene quantum dot, topdown, doping ratio, the specific capacitance
  • 出版物名称:   NANOSCALE RESEARCH LETTERS
  • ISSN:   1931-7573 EI 1556-276X
  • 通讯作者地址:   Wuhan Univ Technol
  • 被引频次:   7
  • DOI:   10.1186/s11671-019-3045-4
  • 出版年:   2019

▎ 摘  要

Sulfur, nitrogen co-doped graphene quantum dots (S, N-GQDs) with high crystallinity were obtained by a top-down strategy. The as-prepared S, N-GQDs were investigated and the results indicate that S, N-GQDs exhibit a transverse dimension about 20nm and a topographic height of 1-2 layers graphene. The incorporation of S, N can effectively reduce the layers of GQDs and strip the graphene sheets. Moreover, the S, N-GQDs reveal an absorption band located at 405nm and exhibit an adjustable fluorescence characteristic in the excitation-visible range. Meanwhile, the S, N-GQDs shows a high specific capacitance of 362.60Fg(-1) at a fixed scan rate of 5mVs (-1). This high performance is ascribed to the additional high pseudocapacitance provided by the doped S, N and the doping state acting as a trap state to enhance the charge storage capacity. The high specific capacitance advantages of S, N-GQDs illustrate their potential prospects in the capacitors.