• 文献标题:   Laser-induced graphene via the far-infrared irradiation of polyimide films for flexible electric heater applications
  • 文献类型:   Article
  • 作  者:   TSENG SF, TSAI YS
  • 作者关键词:   ultravioletlaserinduced graphene, farinfrared irradiation, flexible electric heater, photothermal, photochemical reaction, graphenization, surface laser fluence
  • 出版物名称:   INTERNATIONAL JOURNAL OF ADVANCED MANUFACTURING TECHNOLOGY
  • ISSN:   0268-3768 EI 1433-3015
  • 通讯作者地址:  
  • 被引频次:   3
  • DOI:   10.1007/s00170-022-09100-8 EA MAR 2022
  • 出版年:   2022

▎ 摘  要

This study investigated ultraviolet-laser-induced graphene (ULIG) through the far-infrared irradiation (FIR) of polyimide films for constructing flexible electric heaters. Graphene, which has a uniform micro-scale porous structure with high electrical conductivity, was formed along the laser-induced paths through photothermal and photochemical reactions. Raman spectroscopy, X-ray diffraction, and X-ray photoelectron spectroscopy were used to measure the microstructure, elemental composition, and chemical states of the ULIG films and thereby investigate their graphenization and defect level. Moreover, the surface morphology and electrical properties of the ULIG films were evaluated using a field-emission scanning electron microscope and source measurement unit, respectively. Finally, optimal processing parameters, namely a surface laser fluence of 48 J/cm(2), a pulse repetition rate of 100 kHz, and a scan pitch of 0.01 mm, were used to fabricate ULIG heaters with triangular and honeycomb electrode structures. The ULIG films with FIR exhibited a high-quality and high-integrity porous structure, a low electrical resistance of 2.55 omega, and a low sheet resistance of 14.34 +/- 2.04 omega/sq. Furthermore, the ULIG heaters exhibited ultrafast heating and cooling rates (90.93 and 89.37 celcius/s, respectively) as well as excellent heating stability and flexibility.