• 文献标题:   Design and synthesis of Z-scheme LaFeO3/MoS2/graphene heterojunction with enhanced photocatalytic performance
  • 文献类型:   Article
  • 作  者:   HUANG LZ, BAO JY, QUAN W, LI XY, ZHAO TT, NING YQ, LU WT, LIU KH, REN FY, TIAN HW
  • 作者关键词:   perovskite oxide, mos2, graphene cocatalyst, zscheme heterojunction, synergistic effect, degradation dye
  • 出版物名称:   JOURNAL OF ALLOYS COMPOUNDS
  • ISSN:   0925-8388 EI 1873-4669
  • 通讯作者地址:  
  • 被引频次:   6
  • DOI:   10.1016/j.jallcom.2022.167948 EA NOV 2022
  • 出版年:   2023

▎ 摘  要

Photocatalysis is an effective way to treat industrial wastewater. Therefore, the design of low-cost and high -activity photocatalysts is crucial for environmental remediation. Herein, a ternary Z-Scheme LaFeO3/MoS2/ graphene nanocomposite photocatalyst was synthesized by a facile two-step hydrothermal approach and tested for the degradation of dye wastewater. To this end, graphene was employed as a substrate for loading LaFeO3 nanospheres and MoS2 nanosheets to act as an electron migration medium for Z-scheme hetero-junction. The obtained LaFeO3/MoS2/graphene photocatalyst showed high efficiency and stable perfor-mance toward the degradation of methylene blue (MB), estimated to 16.5-fold higher than that of sole LaFeO3. The enhanced photocatalytic activity was mainly attributed to the synergistic effect between LaFeO3 and MoS2/graphene co-catalyst, leading to the expansion of the visible light absorption range and opti-mization of the redox potential. Most importantly, the closely contacted Z-scheme heterojunction interface between LaFeO3 and MoS2/graphene facilitated the separation and transport efficiency of photogenerated carriers, as well as prolonged the lifetime of photogenerated carriers. In sum, these results look promising for the future design of highly efficient LaFeO3-based photocatalysts with Z-scheme heterojunction struc-tures.(c) 2022 Elsevier B.V. All rights reserved.