• 文献标题:   Resonance energy transfer from moire-trapped excitons in MoSe2/WSe2 heterobilayers to graphene: Dielectric environment effect
  • 文献类型:   Article
  • 作  者:   HICHRI A, AMAND T, JAZIRI S
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW MATERIALS
  • ISSN:   2475-9953
  • 通讯作者地址:  
  • 被引频次:   1
  • DOI:   10.1103/PhysRevMaterials.5.114002
  • 出版年:   2021

▎ 摘  要

Moire excitons in twisted heterobilayer (HBL) transition metal dichalcogenides (TMDs) exhibit an interesting platform for engineering optical properties. The screening from the dielectric environment surrounding the HBL and the twist angle, arising from vertically stacking two layered TMD materials, allow the possibility to control and tune the interlayer exciton states. In this paper, we show in the first part that interlayer excitons in MoSe2/WSe2 HBL localize due to the moire potential arising within the TMD HBL and discuss the conditions for which each localization site can be viewed as a local quantum emitter. In the second part, we show that the trapped exciton energy can be transferred, via the Forster resonance energy transfer (FRET) mechanism, to an adjacent two-dimensional sheet of doped graphene (Gr). The analysis of the localized exciton quenching rate is provided within the random-phase approximation, which allows one to access the collective electronic behavior within the Gr layer. Our model demonstrates the high sensitivity of FRET efficiency to external parameters, particularly the dielectric environment and the distance between the donor-here the HBL-and the acceptor (Gr). These properties show that FRET can be quite a useful tool for applications in biological systems and nanoscale sensors.