• 文献标题:   High-Performance Ge Quantum Dot Decorated Graphene/Zinc-Oxide Heterostructure Infrared Photodetector
  • 文献类型:   Article
  • 作  者:   LIU X, JI XB, LIU MJ, LIU NZ, TAO Z, DAI Q, WEI L, LI C, ZHANG XB, WANG BP
  • 作者关键词:   germanium quantum dot, infrared photodector, flexible, micronsize device, graphene/zincoxide heterostructure
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244 EI 1944-8252
  • 通讯作者地址:   Natl Ctr Nanosci Technol
  • 被引频次:   31
  • DOI:   10.1021/am5072173
  • 出版年:   2015

▎ 摘  要

A novel size-controllable germanium quantum dot (Ge QD) is synthesized and decorated onto reduced graphene oxide (RGO) fragments to overcome the low infrared (IR) photoresponses (similar to 0.1 A/W)(13,14) of pristine graphene. With the integration of flexible substrate, monolayer graphene (MLG) electrode and n-type zinc oxide (ZnO), a high-performance QD-decorated-RGO/ZnO heterostructure infrared photodetector is reported in this study. The Ge QD-decorated-RGO hybrid photosensitive composite improves the responsivity (similar to 9.7 A/W, 1400 nm) in IR waveband without sacrificing the response speed (similar to 40 mu s rise time and 90 mu s recovery time). In addition, the effective barrier formed between graphene and ZnO interface restricts the dark current (similar to 1.4 nA, -3 V) to guarantee the relatively excellent rectifying behavior and high on/off ratio (similar to 10(3)) for this IR photodetector. With these superior inherent properties and micron-sized sensing active area, this photodetector manifests great potential in the future application of graphene-based IR photodetector.