• 文献标题:   Highly Sensitive Humidity Sensor Based on Freestanding Graphene Oxide Sheets for Respiration and Moisture Detection
  • 文献类型:   Article
  • 作  者:   TRIPATHI D, TRIPATHI S, RAWAT RK, CHAUHAN P
  • 作者关键词:   graphene oxide, humidity sensor, modified hummers method, functional group
  • 出版物名称:   JOURNAL OF ELECTRONIC MATERIALS
  • ISSN:   0361-5235 EI 1543-186X
  • 通讯作者地址:  
  • 被引频次:   2
  • DOI:   10.1007/s11664-022-10186-9 EA JAN 2023
  • 出版年:   2023

▎ 摘  要

Graphene oxide (GO) is regarded as one of the best materials for humidity sensing owing to its unique structure (defect enriched) and excellent adsorption properties. Herein, GO was prepared by modified Hummers' method for the fabrication of highly sensitive humidity sensors. The strong diffraction peak at 10.06 degrees in the x-ray diffraction (XRD) pattern and increased I-D/I-G ratio (0.96) for GO obtained from Raman spectroscopy indicate the formation of GO. The Brunauer-Emmett-Teller (BET) analysis for GO revealed a surface area of 17 m(2)/g and a pore radius of 20 A. The surface morphology and topography of GO sheets were examined by field emission scanning electron microscopy, transmission electron microscopy and atomic force microscopy, respectively. For humidity sensing application, a device was prepared by drop casting of GO on interdigitated electrodes and its sensitivity was investigated at room temperature (26 degrees C) under a different relative humidity (RH) level of 11-97% RH. The GO sensor exhibited high sensing response at 11-97-11% RH with good response (13 s)/recovery time (32 s). Notably, the sensor displayed very small humidity hysteresis (0.26%), excellent repeatability and long-term stability (1.13% decrease). Moreover, the proposed sensor quickly responded to different human respiration including nose breath, normal/fast (exercise) mouth breathing, and human skin moisture (sweat) as well as simple spoken words. This finding indicates that flexible, freestanding GO sheets have broad applications in smart humidity sensing devices and medical care treatment.