• 文献标题:   Construction of a hybrid graphene oxide/nanofibrillated cellulose aerogel used for the efficient removal of methylene blue and tetracycline
  • 文献类型:   Article
  • 作  者:   WANG ZG, SONG L, WANG YQ, ZHANG XF, YAO JF
  • 作者关键词:   aerogel, cellulose, exfoliation, graphene oxide, pipi interaction
  • 出版物名称:   JOURNAL OF PHYSICS CHEMISTRY OF SOLIDS
  • ISSN:   0022-3697 EI 1879-2553
  • 通讯作者地址:  
  • 被引频次:   40
  • DOI:   10.1016/j.jpcs.2020.109839 EA JAN 2021
  • 出版年:   2021

▎ 摘  要

A composite graphene oxide (GO)/nanocellulose aerogel was prepared by dispersing cellulose nanofibrils (CNFs) into GO nanosheets. CNFs with high aspect ratios and negative potential helped the exfoliation of GO flakes without the need of a chemical linker via steric hindrance and electrostatic repulsion. Water purification tests were performed using methylene blue (MB) and tetracycline (TC) as model pollutants. The composite aerogel obeyed a pseudo-second-order model and Langmuir adsorption isotherm. The composite aerogel possesses a maximum adsorption capacity of 111.2 mg/g for MB and 47.3 mg/g for TC. Meanwhile, the aerogel can be easily recycled and regenerated using ethanol. After three cycles, the aerogel can maintain a high removal efficiency for MB (98%) and TC (97%). The adsorption mechanism was mainly ascribed to electrostatic attraction and pi-pi interactions.