• 文献标题:   Centimeter-Sized Monolayer CVD Graphene with High Power Factor for Scalable Thermoelectric Applications
  • 文献类型:   Article
  • 作  者:   SCHRADE M, XING W, THORSHAUG K, BELLE BD
  • 作者关键词:   graphene, electrostatic doping, thermoelectric, ionic gel, ferroelectric
  • 出版物名称:   ACS APPLIED ELECTRONIC MATERIALS
  • ISSN:  
  • 通讯作者地址:  
  • 被引频次:   2
  • DOI:   10.1021/acsaelm.1c00995
  • 出版年:   2022

▎ 摘  要

Among the many extraordinary qualities of graphene, its thermoelectric properties have attracted significant interest, for example, in active cooling applications. Here, we report on the thermoelectric transport properties of centimeter-sized monolayer CVD graphene, electrostatically controlled by a high-capacity ionic gel. The power factor reaches 7 and 5.4 mW m(-1) K-2 for hole and electron conduction, respectively, similar to earlier reports obtained for microdevices despite our devices being over 2 orders of magnitude larger. On the basis of these results, we propose nonvolatile ferroelectric polarization as a scalable technology for graphene-based thermoelectric applications.