• 文献标题:   Transparent, Flexible, All-Reduced Graphene Oxide Thin Film Transistors
  • 文献类型:   Article
  • 作  者:   HE QY, WU SX, GAO S, CAO XH, YIN ZY, LI H, CHEN P, ZHANG H
  • 作者关键词:   reduced graphene oxide, fieldeffect transistor, protein detection, nanoelectronic sensing
  • 出版物名称:   ACS NANO
  • ISSN:   1936-0851 EI 1936-086X
  • 通讯作者地址:   Nanyang Technol Univ
  • 被引频次:   222
  • DOI:   10.1021/nn201118c
  • 出版年:   2011

▎ 摘  要

Owing to their unique thickness-dependent electronic properties, together with perfect flexibility and transparency, graphene and its relatives make fantastic material for use in both active channel and electrodes In various electronic devices. On the other hand, the electronic sensors based on graphene show high potential in detection of both chemical and biological species with high sensitivity. In this contribution, we report the fabrication of all-reduced graphene oxide (rGO) thin film transistors by a combination of solution-processed rGO electrodes with a micropatterned rGO channel, and then study their applications in biosensing. Our all-rGO devices are cost-effective, highly reproducible, and reliable. The fabricated electronic sensor Is perfectly flexible with high transparency, showing good sensitivity in detecting proteins in the physiological buffer. As a proof of concept, fibronectin as low as 0.5 nM was successfully detected, which is comparable with the previously reported protein sensors based on single-layer pristine graphene obtained from mechanical deavage. The specific detection of avidin by using biotinylated all-rGO sensor Is also successfully demonstrated.