• 文献标题:   Ultrasensitive photodetectors based on graphene quantum dot-InSe mixed-dimensional van der Waals heterostructures
  • 文献类型:   Article
  • 作  者:   SONG S, QIAO J, SHEN MY, ZHANG GP, FENG F, SOMEKH MG
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS CHEMISTRY C
  • ISSN:   2050-7526 EI 2050-7534
  • 通讯作者地址:  
  • 被引频次:   3
  • DOI:   10.1039/d2tc03395j EA NOV 2022
  • 出版年:   2022

▎ 摘  要

Two-dimensional (2D) semiconducting materials like InSe have attracted considerable attention in the photoelectric detection field due to their outstanding properties, such as a large tunable bandgap, high carrier mobility, low electron effective mass and high absorption coefficient. In this work, a mixed-dimensional van der Waals heterostructure (MvdWH)-based photodetector combining graphene quantum dots (GQDs) with InSe was fabricated. The GQD/InSe MvdWH photodetector achieved a high responsivity of 27.48 A W-1 and a large detectivity of 1.2 x 10(12) Jones at 635 nm, a sixty-fold increase compared to the pure InSe devices. The significant enhancement in photoresponsive performances can be attributed to the p-type doping effect and efficient charge transfer from GQDs to InSe. The novel 0D/2D van der Waals heterojunctions offer tremendous opportunities in high-performance photodetectors.