• 文献标题:   Amino-functionalized graphene oxide blend with monoethanolarnine for efficient carbon dioxide capture
  • 文献类型:   Article
  • 作  者:   SONG YT, CAO LD, YU J, ZHANG SJ, CHEN SM, JIANG Y
  • 作者关键词:   graphene oxide, carbon dioxide, aminefunctionalized, absorption performance
  • 出版物名称:   JOURNAL OF ALLOYS COMPOUNDS
  • ISSN:   0925-8388 EI 1873-4669
  • 通讯作者地址:   Chinese Acad Sci
  • 被引频次:   10
  • DOI:   10.1016/j.jallcom.2017.01.310
  • 出版年:   2017

▎ 摘  要

In this work, we have developed a highly efficient approach to fabricating graphene oxide (GO) functionalized with melamine molecule by chemical crosslinking. The melamine-functionalized graphene oxide (MEL-GO) was characterized by FT-IR, Raman, XRD TGA, XPS, SEM and TEM. Using monoethanolamine (MEA) aqueous solution as the basic absorbent, The absorbance performance of CO2 in the (MEL-GO)+MEA-FH2O solid-liquid hybrid absorbent for different mass concentrations of MEL-GO in 30 wt% MEA aqueous solution was investigated. The solubility of CO2 in (MEL-GO)+MEA+H2O absorbents is much larger than that in 30 wt% MEA aqueous solution. Moreover, when the partial pressure of CO2 continues to go up, the solubility of CO2 was obviously increased with increasing mass concentrations of MEL-GO. The results suggest that MEL-GO is beneficial to enhance the solubility of CO2 in MEA aqueous solution. (C) 2017 Elsevier B.V. All rights reserved.