• 文献标题:   Improved photoelectrocatalytic degradation of tetrabromobisphenol A with silver and reduced graphene oxide-modified TiO2 nanotube arrays under simulated sunlight
  • 文献类型:   Article
  • 作  者:   ZHOU QX, WANG MY, TONG YY, WANG HY, ZHOU XQ, SHENG XY, SUN Y, CHEN CM
  • 作者关键词:   photoelectrocatalysi, tetrabromobisphenol a, tio2 nanotube array, reductive graphene oxide modified tio2, nanotube array, reductive graphene oxide sliver, nanoparticles comodified tio2 nanotube, array
  • 出版物名称:   ECOTOXICOLOGY ENVIRONMENTAL SAFETY
  • ISSN:   0147-6513 EI 1090-2414
  • 通讯作者地址:   China Univ Petr
  • 被引频次:   6
  • DOI:   10.1016/j.ecoenv.2019.109472
  • 出版年:   2019

▎ 摘  要

In present study, reductive graphene oxide and silver nanoparticles co-comodified TiO2 nanotube arrays were prepared, and which was investigated to degrade tetrabromobisphenol A. The arrays co-modified with silver nanoparticles and reductive graphene oxide prepared by electrodeposition method exhibited good photoelectrocatalytic degradative activity for tetrabromobisphenol A, and the degradation efficiency reached 99.6% within 80 min. The synergistic effect of high photoresponse of Ag nanoparticles with their high capture ability for photogenerated electrons and the extended wavelength absorption range of reductive graphene oxide resulted in the highest degradation efficiencies. Degradation is postulated to follow a stepwise reductive debromination mechanism.