▎ 摘　　要

In this work, sharp wrinkles on graphene films, caused by graphene duplicating the grain boundary cracks of copper foil during the preparation process, were carefully explored. A secondary-transferring graphene film process was proposed to re-transform the Peak morphology of graphene surface into Valley form. The process we have developed is highly effective and almost nondestructive to the graphene through testing the surface morphology and photo-electric properties before and after the secondary-transferring process. Flexible organic light-emitting device (FOLED) with PEDOT:PSS/SLG/NOA63 framework as a targeted application was fabricated to illustrate the value of our proposed method in fabricating stable devices, the maximum luminance can reach about 35000cd/m(2), and the maximum current efficiency was 16.19cd/A. This method can also be applied to the roll-to-roll preparation of large area high-quality graphene.