• 文献标题:   Enhancing catalytic performance of Au catalysts by noncovalent functionalized graphene using functional ionic liquids
  • 文献类型:   Article
  • 作  者:   LI SW, GUO SJ, YANG HL, GOU GL, REN R, LI J, DONG ZP, JIN J, MA JT
  • 作者关键词:   au nanoparticle, 3 4 9 10perylene tetracarboxylic acid, ionic liquid, noncovalent functionalized grapheme, supported catalyst
  • 出版物名称:   JOURNAL OF HAZARDOUS MATERIALS
  • ISSN:   0304-3894 EI 1873-3336
  • 通讯作者地址:   Lanzhou Univ
  • 被引频次:   51
  • DOI:   10.1016/j.jhazmat.2014.01.033
  • 出版年:   2014

▎ 摘  要

New catalyst, prepared through Au nanoparticles anchored on the Ionic Liquid of 3,4,9,10-perylene tetracarboxylic acid-noncovalent functionalized graphene (Au/PDIL-GS), was fabricated using a facile and environment-friendly approach. The information of the morphologies, sizes, dispersion of Au nanoparticles (NPs) and chemical composition for the as-prepared catalysts was verified by systematic characterizations, including transmission electron microscopy (TEM), high-resolution transmission electron microscopy (HRTEM), Raman spectra, X-ray diffraction (XRD) and X-Ray photoelectron spectroscopy (XPS). As a new catalyst, the resulting Au/PDIL-GS exhibited excellent catalytic activity in the reduction of 4-nitrophenol because of the synergistic effect between the PDIL-GS and Au NPs. The facile and environment-friendly approach provides a green way to effectively synthesize low cost Au-based catalysts for 4-NP reduction and is promising for the development of other useful materials. (C) 2014 Elsevier B.V. All rights reserved.