• 文献标题:   One-step synthesis of annual ring-shaped planar nitrogen/sulfur co-doped nanoporous graphene for supercapacitance
  • 文献类型:   Article
  • 作  者:   LIANG J, SHAN Q, LIU TQ, LIANG WB, ZHANG X, QI W, TAN HX, DU SB, QIAN LJ, LI Z, CHEN XM
  • 作者关键词:   annual ringshaped, nitrogen/sulfur doped, nanoporous graphene, supercapacitance
  • 出版物名称:   ELECTROCHIMICA ACTA
  • ISSN:   0013-4686 EI 1873-3859
  • 通讯作者地址:  
  • 被引频次:   6
  • DOI:   10.1016/j.electacta.2021.139137 EA SEP 2021
  • 出版年:   2021

▎ 摘  要

Heteroatom-doped nanoporous graphene has great potential as emerging energy storage materials, but the complex synthetic routes and disordered structure limit the improvement of supercapacitance per-formance. Herein, we develop a one-step synthesis strategy to obtain nitrogen/sulfur doped nanoporous graphene (NS-NG). Graphene oxides absorbed with dyes are burned in a confined interlayer of porous hy-drotalcite for preparing NS-NG. Interestingly, the NS-NG retains the morphology of multilayer graphene oxides coated with fiber rods before combustion, so it exhibits the annual ring-shaped structure, larger surface area, and highly porosity. Importantly, the NS-NG not only shows a high specific capacitance of 325 F g(-1), and also has a high energy density of 25 Wh kg(-1) at a high power density of 1906 W kg(-1) with an excellent capacity retention of 86% after 10,000 cycles applied in the two-electrode symmetric super-capacitor at a current density of 2 A g(-1) in 0.5 M Na2SO4 aqueous solution. (C) 2021 Elsevier Ltd. All rights reserved.