• 文献标题:   Energy flows in graphene: hot carrier dynamics and cooling
  • 文献类型:   Article
  • 作  者:   SONG JCW, LEVITOV LS
  • 作者关键词:   lightmatter interaction, electronlattice cooling, supercollision
  • 出版物名称:   JOURNAL OF PHYSICSCONDENSED MATTER
  • ISSN:   0953-8984 EI 1361-648X
  • 通讯作者地址:   CALTECH
  • 被引频次:   24
  • DOI:   10.1088/0953-8984/27/16/164201
  • 出版年:   2015

▎ 摘  要

Long lifetimes of hot carriers can lead to qualitatively new types of responses in materials. The magnitude and time scales for these responses reflect the mechanisms governing energy flows. We examine the microscopics of two processes which are key for energy transport, focusing on the unusual behavior arising due to graphene's unique combination of material properties. One is hot carrier generation in its photoexcitation dynamics, where hot carriers multiply through an Auger type carrier-carrier scattering cascade. The hot-carrier generation manifests itself through elevated electronic temperatures which can be accessed in a variety of ways, in particular optical conductivity measurements. Another process of high interest is electron-lattice cooling. We survey different cooling pathways and discuss the cooling bottleneck arising for the momentum-conserving electron-phonon scattering pathway. We show how this bottleneck can be relieved by higher-order collisions-supercollisions-and examine the variety of supercollision processes that can occur in graphene.