• 文献标题:   An enhanced ultrasensitive solar-blind UV photodetector based on an asymmetric Schottky junction designed with graphene/beta-Ga2O3/Ag
  • 文献类型:   Article
  • 作  者:   QI S, LIU JH, YUE JY, JI XQ, SHEN JY, YANG YT, WANG JJ, LI S, WU ZP, TANG WH
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS CHEMISTRY C
  • ISSN:   2050-7526 EI 2050-7534
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.1039/d3tc01456h EA MAY 2023
  • 出版年:   2023

▎ 摘  要

Ga2O3 has generated considerable interest as a wide bandgap semiconductor and is used for solar-blind deep ultraviolet photodetectors. Additionally, graphene serving as a transparent electrode material can improve device performance. However, due to defects at the contact interface between graphene and Ga2O3, existing devices based on graphene/Ga2O3 are liable to elevated dark currents. In this work, we constructed a graphene/beta-Ga2O3/Ag asymmetric Schottky junction photodetector, which addresses this issue. Taking advantage of the asymmetric structure design to suppress dark current and the transparent graphene electrode increasing the carrier collection efficiency, the device achieved an outstanding responsivity of 44.09 A W-1, a high detectivity of 5.84 x 10(12) Jones, a remarkable external quantum efficiency of 2.15 x 10(4)%, and a fast response time of 99.60 ms/27.74 ms. More importantly, owing to reverse bias voltage on the high barrier side, it possesses a low dark current of 12.09 pA with a light-to-dark ratio of up to 10(4). All in all, the graphene/beta-Ga2O3/Ag asymmetric Schottky junction photodetector has considerable potential as a deep ultraviolet detector.