• 文献标题:   Fabrication of BiOBr/MoS2/graphene oxide composites for efficient adsorption and photocatalytic removal of tetracycline antibiotics
  • 文献类型:   Article
  • 作  者:   LI YH, LAI Z, HUANG ZJ, WANG HY, ZHAO CX, RUAN GH, DU FY
  • 作者关键词:   biobr, mos2/go, adsorption, photocatalytic degradation, antibiotics removal
  • 出版物名称:   APPLIED SURFACE SCIENCE
  • ISSN:   0169-4332 EI 1873-5584
  • 通讯作者地址:  
  • 被引频次:   49
  • DOI:   10.1016/j.apsusc.2021.149342 EA FEB 2021
  • 出版年:   2021

▎ 摘  要

Bismuth oxybromide/molybdenum disulfide/graphene oxide (BiOBr/MoS2/GO) heterojunction composites were fabricated to modulate the adsorption ability and photocatalytic degradation performance toward oxytetracycline (OTC). The flowerlike BiOBr/MoS2/GO composites demonstrated excellent photocatalytic activies for the OTC degradation. Specifically, OTC, tetracycline, chlorotetracycline, and doxycycline were simultaneously removed with degradation rates higher than 98% under visible light irradiation within 40 min. Radical trapping experiments indicated that photogenerated holes (h(+)), hydroxyl radicals ((OH)-O-center dot), and superoxide radicals (O-center dot(2-)) played crucial roles in photocatalytic OTC degradation. Further, Possible transformation pathway and photocatalytic mechanism were proposed by investigating the intermediates in OTC degradation process.