• 文献标题:   Preparation of Ag(Au)/Graphene-TiO2 Composite Photocatalysts and Their Catalytic Performance under Simulated Sunlight Irradiation
  • 文献类型:   Article
  • 作  者:   JIANG LX, LI KX, YAN LS, DAI YH, HUANG ZM
  • 作者关键词:   graphene, titania, silver, gold, solvothermal reduction, photoreduction, rhodamine b, methyl orange
  • 出版物名称:   CHINESE JOURNAL OF CATALYSIS
  • ISSN:   0253-9837
  • 通讯作者地址:   Nanchang Hangkong Univ
  • 被引频次:   13
  • DOI:   10.3724/SP.J.1088.2012.20820
  • 出版年:   2012

▎ 摘  要

To improve the solar utilization efficiency of TiO2, the graphene-TiO2 and Ag(Au)/graphene-TiO2 composite photocatalysts were prepared by solvothermal reduction and photoreduction deposition technique, respectively. The phase structure, morphology, porosity, optical absorption property as well as composition and structure of as-prepared materials were characterized. The results indicated that TiO2 interacts with graphene via Ti-O-C covalent bonds and Ag or Au nano-particles evenly deposite on the graphene and TiO2 surface. The photocatalytic activity and degradation kinetics of the as-prepared photocatalysts were studied by the degradation of aqueous rhodamine B and methyl orange under solar simulating Xe lamp irradiation. The results indicated that the composite photocatalysts exhibit higher photocatalytic activity compared with pure TiO2 due to enhanced quantum efficiency, narrowed band gap, and perfect textural properties.