• 文献标题:   Femtosecond Population Inversion and Stimulated Emission of Dense Dirac Fermions in Graphene
  • 文献类型:   Article
  • 作  者:   LI T, LUO L, HUPALO M, ZHANG J, TRINGIDES MC, SCHMALIAN J, WANG J
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW LETTERS
  • ISSN:   0031-9007 EI 1079-7114
  • 通讯作者地址:   Iowa State Univ
  • 被引频次:   157
  • DOI:   10.1103/PhysRevLett.108.167401
  • 出版年:   2012

▎ 摘  要

We show that strongly photoexcited graphene monolayers with 35 fs pulses quasi-instantaneously build up a broadband, inverted Dirac fermion population. Optical gain emerges and directly manifests itself via a negative conductivity at the near-infrared region for the first 200 fs, where stimulated emission completely compensates absorption loss in the graphene layer. Our experiment-theory comparison with two distinct electron and hole chemical potentials reproduce absorption saturation and gain at 40 fs, revealing, particularly, the evolution of the transient state from a hot classical gas to a dense quantum fluid with increasing the photoexcitation.