• 文献标题:   Particulate Matter Capturing via Naturally Dried ZIF-8/Graphene Aerogels under Harsh Conditions
  • 文献类型:   Article
  • 作  者:   MAO JJ, TANG YX, WANG YD, HUANG JY, DONG XL, CHEN Z, LAI YK
  • 作者关键词:  
  • 出版物名称:   ISCIENCE
  • ISSN:  
  • 通讯作者地址:   Fuzhou Univ
  • 被引频次:   16
  • DOI:   10.1016/j.isci.2019.05.024
  • 出版年:   2019

▎ 摘  要

Particulate matter (PM) pollution poses a serious threat to the environment and public health. Capture of PM is best performed at the emission source, such as car exhaust exit points, although it is a challenge for filters to work under harsh conditions of high temperatures and flow rate. Here we designed a thermally stable PM filter by in situ anchoring of zeolite imidazole framework-8 (ZIF-8) on a three-dimensional (3D) network of reduced graphene oxide aerogel (rGA) through natural drying. Owing to high specific surface area, well-connected porous network of graphene aerogel, and large number of metal sites from ZIF-8/rGA, the capture efficiencies for PM(2.5 )and PM10 are over 99.3% and 99.6%, respectively, at ambient conditions, and the efficiencies remain high in harsh conditions (PM2.5 and PM10 : >98.8% and >99.1%, respectively, at 200 degrees C at a flow velocity of 30 L/min). The filter can be regenerated by a simple washing process.