• 文献标题:   Biexciton Auger Recombination in Colloidal Graphene Quantum Dots
  • 文献类型:   Article
  • 作  者:   SUN C, FIGGE F, MCGUIRE JA, LI QQ, LI LS
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW LETTERS
  • ISSN:   0031-9007 EI 1079-7114
  • 通讯作者地址:   Michigan State Univ
  • 被引频次:   14
  • DOI:   10.1103/PhysRevLett.113.107401
  • 出版年:   2014

▎ 摘  要

We measure biexciton Auger recombination (AR) in colloidal graphene quantum dots (GQDs) by transient absorption spectroscopy. AR is reflected in GQDs with 132 and 168 sp(2)-hybridized C atoms as a decay with a similar to 0.3 ps time constant and an amplitude depending superlinearly on pump fluence. Despite the orders-of-magnitude difference in size between GQDs and carbon nanotubes, their biexciton AR rates are similar. This similarity is a result of strong carrier interactions in sp(2)-hybridized carbon nanostructures and suggests that GQDs may hold promise in the context of carrier multiplication.