• 文献标题:   Optical-Phonon Resonances with Saddle-Point Excitons in Twisted-Bilayer Graphene
  • 文献类型:   Article
  • 作  者:   JORIO A, KASPERCZYK M, CLARK N, NEU E, MALETINSKY P, VIJAYARAGHAVAN A, NOVOTNY L
  • 作者关键词:   graphene, raman scattering, optical reflectivity, coherence
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   ETH
  • 被引频次:   21
  • DOI:   10.1021/nl502412g
  • 出版年:   2014

▎ 摘  要

Twisted-bilayer graphene (tBLG) exhibits van Hove singularities in the density of states that can be tuned by changing the twisting angle theta. A theta-defined tBLG has been produced and characterized with optical reflectivity and resonance Raman scattering. The theta-engineered optical response is shown to be consistent with persistent saddle-point excitons. Separate resonances with Stokes and anti-Stokes Raman scattering components can be achieved due to the sharpness of the two-dimensional saddle-point excitons, similar to what has been previously observed for one-dimensional carbon nanotubes. The excitation power dependence for the Stokes and anti-Stokes emissions indicate that the two processes are correlated and that they share the same phonon.