• 文献标题:   Highly Efficient Photocatalytic Disinfection of Escherichia coli by Rose Bengal-Functionalized Graphene Oxide Nanosheets
  • 文献类型:   Article
  • 作  者:   CHI FP, CHEN PP, MAO CJ
  • 作者关键词:   graphene oxide, rose bengal, reactive oxygen specie, sterilization
  • 出版物名称:   JOURNAL OF NANOSCIENCE NANOTECHNOLOGY
  • ISSN:   1533-4880 EI 1533-4899
  • 通讯作者地址:   Anhui Univ
  • 被引频次:   0
  • DOI:   10.1166/jnn.2020.18615
  • 出版年:   2020

▎ 摘  要

Rose Bengal (RB) was used as a functional pigment and poly dimethyl diallyl ammonium chloride was used as a coupling agent to modify Graphene Oxide (GO) in order to enhance the light absorption and ROS generation of GO. GO, RB and the obtained RB-PDDA-GO were characterized by scanning electron microscopy, transmission electron microscopy, Fourier transform infrared spectrometry, thermogravimetric analysis, Raman spectroscopy, UV-visible spectrophotometry, and X-ray photoelectron spectroscopy. The oxidation of hydroquinone to p-benzoquinone was used to evaluate the oxidation ability. Three kinds of reactive oxygen species (O-2(center dot-), O-1(2) and center dot OH) produced by the materials under light irradiation were detected by the ESR method using TEMP (2,2,6,6-tetramethyl-4-piperidine) and DMPO (5,5-dimethyl-1-pyrroline-N-oxide) as capture agents. The results showed that RB-PDDA-GO produced more ROS under light than GO. Antibacterial experiments were carried out with E. coli as the target strain to detect the actual utility of ROS produced by the materials. The results showed that RB-PDDA-GO had a significant sterilization effect.