• 文献标题:   Reduced graphene oxide/carbon nitride composite sponge for interfacial solar water evaporation and wastewater treatment
  • 文献类型:   Article
  • 作  者:   ZHANG H, LI LL, GENG L, TAN XY, HU YX, MU P, LI J
  • 作者关键词:   reduced graphene oxide, composite sponge, photothermal conversion, photocatalysi, water evaporation
  • 出版物名称:   CHEMOSPHERE
  • ISSN:   0045-6535 EI 1879-1298
  • 通讯作者地址:  
  • 被引频次:   2
  • DOI:   10.1016/j.chemosphere.2022.137163 EA NOV 2022
  • 出版年:   2023

▎ 摘  要

Interfacial solar-driven steam generation has been proposed as a cost-effective green sustainable technology to alleviate the freshwater crisis. However, the desire to produce clean water from water sources containing organic contaminants is still remains a challenge due to the limitations of the traditional wastewater treatment methods. Here, we constructed a g-C3N4-based composite sponge solar steam generator (rGCPP) by a simple hydrothermal reaction. Benefiting from its low cost and easy preparation, this evaporator can be expected to be a promising candidate for the alleviation of water shortages and water pollution in practical applications. By combination of the solar steam generation and the photocatalysis into the rGCPP-based interfacial solar-driven steam generation system, the resulted rGCPP-based solar steam generator performs outstanding solar absorption of 90.8%, which achieves high evaporation rate of 1.875 kg m(-2) h(-1) and solar-to-vapor efficiency of 81.07% under 1 sun irradiation. Meanwhile, organic pollutants in the water source can be completely removed by photocatalytic degradation and the degradation rates were measured to be 99.20% for methylene blue and 91.07% for rhodamine B, respectively. Consequently, the as-prepared composite sponge has promising applications in generating clean water and alleviating water pollution.