• 文献标题:   High-Temperature Structural Stability of Intercalated Cerium Superhydride into Graphene Sheets at Low Pressure
  • 文献类型:   Article
  • 作  者:   RASTKHADIV MA
  • 作者关键词:   hightemperature, structural, stability, superhydride, graphene
  • 出版物名称:   JOURNAL OF SUPERCONDUCTIVITY NOVEL MAGNETISM
  • ISSN:   1557-1939 EI 1557-1947
  • 通讯作者地址:  
  • 被引频次:   1
  • DOI:   10.1007/s10948-022-06332-3 EA JUL 2022
  • 出版年:   2022

▎ 摘  要

Finding high-temperature superconductors has been one of the main challenges of condensed matter physics. Recent progress in this regard includes the reports of room-temperature superconductivity in carbonaceous sulfur hydride. However, this superconductivity is strongly restricted by an extremely high-pressure condition (similar to 100GPa) that makes it difficult to apply in technology and industry. Therefore, the cuprate materials with T-c = 133.5 K are considered as the highest temperature superconductors at low pressures. The main purpose of the present work is to open doors toward finding high-temperature superconductivity at low pressure. For this purpose, we consider two graphene layers with sine form corrugations where their honeycomb patterns are exactly on top of each other with some doped molecules placed between them. We consider H2S, H3S, and CeH9 as doped molecules, separately. Employing the lowest-order constrained variational method, we calculate thermodynamic quantities of the system. Based on pressure-density and magnetic susceptibility diagrams of the system, we observe a second-order phase transition at T-c = 186.3 K and P-c = 2.35 K.angstrom(-3) for valence electrons with CeH9 doped molecules. Meanwhile, no phase transition occurs for H2S and H3S at T > 133.5 K. The novel result of this paper is the prediction of a critical temperature which is approximately 53 K greater than the cuprate materials without applying the external pressure.