• 文献标题:   Low-Temperature Graphene Growth by Forced Convection of Plasma-Excited Radicals
  • 文献类型:   Article
  • 作  者:   KIM J, SAKAKITA H, ITAGAKI H
  • 作者关键词:   graphene, forced convection plasma cvd, lowtemperature growth, selflimiting growth
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   Natl Inst Adv Ind Sci Technol
  • 被引频次:   8
  • DOI:   10.1021/acs.nanolett.8b03769
  • 出版年:   2019

▎ 摘  要

We developed the forced convection (FC)-PECVD method for the synthesis of graphene, in which a specially designed blowing plasma source is used at moderate gas pressure (1-10 Torr) and the distribution of reactive radicals reaching the substrate surface can be controlled by forced convection. Self-limiting growth of graphene occurs on copper foil, and monolayer graphene growth with a few defects is achieved even at low temperatures (<400 degrees C). We also demonstrated the enlargement of the growth area using the scalable blowing plasma source. We expect that the FC-PECVD method overcomes the limitations of conventional low-temperature PECVD and provides a breakthrough for the achievement of industrial applications based on graphene.