• 文献标题:   Microstructure and electrothermal characterization of transparent reduced graphene oxide thin films manufactured by spin-coating and thermal reduction
  • 文献类型:   Article
  • 作  者:   KIM SY, GANG H, PARK GT, JEON H, JEONG YG
  • 作者关键词:   reduced graphene oxide, thin film, spincoating, thermal reduction, electrothermal property
  • 出版物名称:   RESULTS IN PHYSICS
  • ISSN:   2211-3797
  • 通讯作者地址:  
  • 被引频次:   7
  • DOI:   10.1016/j.rinp.2021.104107 EA APR 2021
  • 出版年:   2021

▎ 摘  要

We herein report the microstructure, optical and electrothermal properties of a series of reduced graphene oxide (RGO) thin films, which are manufactured by spin-coating (1 and 3 layers) of graphene oxide (GO) dispersion on a quartz substrate and thermal reduction at different temperatures of 800-1000 degrees C. The energy dispersive X-ray spectra reveal that the relative carbon content of RGO films increases from 84.3 at% to 93.5 at% with increasing the thermal reduction temperature from 800 degrees C and 1000 degrees C, whereas the oxygen content decreases from 15.7 at % to 6.5 at%. The optical transmittance of RGO1 (1 spin-coating layer) and RGO3 (3 spin-coating layers) films at 550 nm is characterized 32.7-40.8% and 6.3-12.4%, respectively, although it decreases with increasing the thermal reduction temperature. The sheet resistance of RGO1 films decreases from 5160 Omega/sq to 1220 Omega/sq with the increment of the thermal reduction temperature, whereas the sheet resistance of RGO3 films decreased from 1080 Omega/sq to 350 Omega/sq. The decreases in optical transparency and sheet resistance values of RGO thin films are due to the successful reduction of GO films with oxygen-related functional groups to electrically conductive graphene films during the thermal treatment. The RGO thin films are characterized to exhibit high performance electrothermal behavior in terms of uniform temperature distribution, controllable steady-state saturated temperatures, rapid temperature responsiveness, and electric power efficiency at input power densities.