• 文献标题:   Single-step ambient-air synthesis of graphene from renewable precursors as electrochemical genosensor
  • 文献类型:   Article
  • 作  者:   SEO DH, PINEDA S, FANG JH, GOZUKARA Y, YICK S, BENDAVID A, LAM SKH, MURDOCK AT, MURPHY AB, HAN ZJ, OSTRIKOV K
  • 作者关键词:  
  • 出版物名称:   NATURE COMMUNICATIONS
  • ISSN:   2041-1723
  • 通讯作者地址:   CSIRO Mfg
  • 被引频次:   39
  • DOI:   10.1038/ncomms14217
  • 出版年:   2017

▎ 摘  要

Thermal chemical vapour deposition techniques for graphene fabrication, while promising, are thus far limited by resource-consuming and energy-intensive principles. In particular, purified gases and extensive vacuum processing are necessary for creating a highly controlled environment, isolated from ambient air, to enable the growth of graphene films. Here we exploit the ambient-air environment to enable the growth of graphene films, without the need for compressed gases. A renewable natural precursor, soybean oil, is transformed into continuous graphene films, composed of single-to-few layers, in a single step. The enabling parameters for controlled synthesis and tailored properties of the graphene film are discussed, and a mechanism for the ambient-air growth is proposed. Furthermore, the functionality of the graphene is demonstrated through direct utilization as an electrode to realize an effective electrochemical genosensor. Our method is applicable to other types of renewable precursors and may open a new avenue for low-cost synthesis of graphene films.