• 文献标题:   A green route to synthesize nitrogen-enriched graphene-like carbon nanosheets from bio-oil for supercapacitors
  • 文献类型:   Article
  • 作  者:   WANG Q, QIN B, ZHANG XH, WANG Y, JIN LE, CAO Q
  • 作者关键词:   biooil, nitrogenenriched, carbon nanosheet, graphene, supercapacitor
  • 出版物名称:   DIAMOND RELATED MATERIALS
  • ISSN:   0925-9635 EI 1879-0062
  • 通讯作者地址:  
  • 被引频次:   3
  • DOI:   10.1016/j.diamond.2021.108530 EA JUL 2021
  • 出版年:   2021

▎ 摘  要

Two-dimensional carbon materials with the combined characteristics of high surface area, plentiful exposed active sites as well as short ion transport distance, have received great attention for fast charge storage. Herein, an environmentally-friendly method is proposed for the fabrication of nitrogen-enriched graphene-like carbon nanosheet (NCS) from bio-oil by using graphitic carbon nitride (g-C3N4) as a self-sacrificing template and ni-trogen source. Notably, compared with our previous work, the obtained carbon material possesses higher ni-trogen content (8.09 at.%). Meanwhile, the carbon nanosheets have a much thinner thickness (similar to 2.8 nm), large size and high electrical conductivity (85 S m(-1)). Consequently, the energy density of the symmetric super-capacitor displays high energy density of 10.6 W h kg(-1) at a power density of 131.1 W kg(-1) in 1 M H2SO4. This study proposes an eco-friendly and low-cost route for the preparation of graphene-like carbon materials for high-performance supercapacitors.