• 文献标题:   Perovskite Quantum Dot-Reduced Graphene Oxide Superstructure for Efficient Photodetection
  • 文献类型:   Article
  • 作  者:   CHOWDHURY FA, PRADHAN B, DING Y, TOWERS A, GESQUIERE A, TETARD L, THOMAS J
  • 作者关键词:   perovskite, perovskite quantum dot, graphene, reduced graphene oxide, superstructure, photodetector, fast photoresponse, charge transfer
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244 EI 1944-8252
  • 通讯作者地址:   Univ Cent Florida
  • 被引频次:   0
  • DOI:   10.1021/acsami.0c11966
  • 出版年:   2020

▎ 摘  要

High-performance photodetectors require efficient photogeneration and charge transport. Perovskite quantum dots (PQDs) have received enormous interest for applications in optoelectronics due to their high photogeneration efficiency. However, they offer meager carrier transport. Reduced graphene oxide (RGO) exhibits inferior photoresponse compared to materials such as quantum dots. An effective synthesis protocol to grow PQDs from the RGO lattice may facilitate direct charge transfers from PQDs to RGO, which could not be accomplished by mixing individual PQDs with RGO or making a bilayer. At ambient condition, the photodetector fabricated with the PQD-RGO superstructure showed high responsivity of 1.07 x 10(3) A/W, detectivity of 1 x 10(13) Jones as well as sharp switching in the visible wavelength. After 3 months in an unencapsulated sample, the photocurrent was decreased similar to 10% of its initial value while preserving speed and cycle stability at ambient condition.