• 文献标题:   Graphene Nanoarchitectonics: Recent Advances in Graphene-Based Electrocatalysts for Hydrogen Evolution Reaction
  • 文献类型:   Review
  • 作  者:   HUANG HJ, YAN MM, YANG CZ, HE HY, JIANG QG, YANG L, LU ZY, SUN ZQ, XU XT, BANDO Y, YAMAUCHI Y
  • 作者关键词:   electrocatalyst, graphene, hybrid structure, hydrogen evolution reaction, nanoparticle
  • 出版物名称:   ADVANCED MATERIALS
  • ISSN:   0935-9648 EI 1521-4095
  • 通讯作者地址:   Hohai Univ
  • 被引频次:   41
  • DOI:   10.1002/adma.201903415 EA SEP 2019
  • 出版年:   2019

▎ 摘  要

Under the double pressures of both the energy crisis and environmental pollution, the exploitation and utilization of hydrogen, a clean and renewable power resource, has become an important trend in the development of sustainable energy-production and energy-consumption systems. In this regard, the electrocatalytic hydrogen evolution reaction (HER) provides an efficient and clean pathway for the mass production of hydrogen fuel and has motivated the design and construction of highly active HER electrocatalysts of an acceptable cost. In particular, graphene-based electrocatalysts commonly exhibit an enhanced HER performance owing to their distinctive structural merits, including a large surface area, high electrical conductivity, and good chemical stability. Considering the rapidly growing research enthusiasm for this topic over the last several years, herein, a panoramic review of recent advances in graphene-based electrocatalysts is presented, covering various advanced synthetic strategies, microstructural characterizations, and the applications of such materials in HER electrocatalysis. Lastly, future perspectives on the challenges and opportunities awaiting this emerging field are proposed and discussed.