• 文献标题:   Enhanced exciton binding energy, Zeeman splitting and spin polarization in hybrid layered nanosheets comprised of (Cd, Mn)Se and nitrogen-doped graphene oxide: implication for semiconductor devices
  • 文献类型:   Article
  • 作  者:   HALDER O, MALLIK G, SUFFCZYNSKI J, PACUSKI W, VARADWAJ KSK, SATPATI B, RATH S
  • 作者关键词:   semiconductor nanosheet, 2d exciton, photoluminescence, magnetooptical propertie
  • 出版物名称:   NANOTECHNOLOGY
  • ISSN:   0957-4484 EI 1361-6528
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.1088/1361-6528/abfdee
  • 出版年:   2021

▎ 摘  要

The exciton properties of (Cd,Mn)Se-NrGO (nitrogen doped reduced graphene oxide) hybrid layered nanosheets have been studied in a magnetic field up to 10 T and compared to those of (Cd,Mn)Se nanosheets. The temperature dependent photoluminescence reveals the hybridization of inter-band exciton and intra-center Mn transition with enhancement of the binding energy of exciton-Mn hybridized state (80 meV with respect to 60 meV in (Cd,Mn)Se nanosheets) and increase of exciton-phonon coupling strength to 90 meV (with respect to 55 meV in (Cd,Mn)Se nanosheets). The circularly polarized magneto-photoluminescence at 2 K provides evidence for magnetic field induced exciton spin polarization and the realization of excitonic giant Zeeman splitting with g (eff) as high as 165.4 +/- 10.3, much larger than in the case of (Cd,Mn)Se nanosheets (63.9 +/- 6.6), promising for implementation in spin active semiconductor devices.