• 文献标题:   Reduced graphene oxide/Bi4O5Br2 nanocomposite with synergetic effects on improving adsorption and photocatalytic activity for the degradation of antibiotics
  • 文献类型:   Article
  • 作  者:   XU MW, WANG YY, HA EN, ZHANG HJ, LI CY
  • 作者关键词:   photocatalytic degradation, reduced graphene oxide, bibased photocatalyst, antibiotic
  • 出版物名称:   CHEMOSPHERE
  • ISSN:   0045-6535 EI 1879-1298
  • 通讯作者地址:  
  • 被引频次:   23
  • DOI:   10.1016/j.chemosphere.2020.129013
  • 出版年:   2021

▎ 摘  要

A photocatalyst based on the integration of reduced graphene oxide (rGO) with Bi4O5Br2 nanosheets was facilely prepared and was confirmed by transmission electron microscope, scanning electron microscope, X-ray diffraction and Raman spectroscopy. The integration of rGO can effectively improve the adsorption and the photocatalytic properties of Bi4O5Br2 nanosheets towards the target antibiotics under visible light irradiation. rGO/Bi4O5Br2 nanocomposite containing 1.0 wt% of rGO exhibits the optimal adsorption and photocatalytic activity towards ciprofloxacin (CIP), norfloxacin (NOR) and tetracycline (TC). The removal efficiencies of CIP, NOR and TC are 97.6%, 80.7% and 98.7%, which are higher than that obtained with Bi4O5Br2 nanosheets. The capture experiments and ESR data show that center dot O-2(-), OH center dot and h(+) are the main active species that participated in the photodegradation system. This work provides a simple strategy to integrate rGO with BixOyXz (X = Cl, Br, I) nanosheets to construct effective photocatalysts for the degradation of antibiotics. (C) 2020 Elsevier Ltd. All rights reserved.