• 文献标题:   Geometric effect of high-resolution electron energy loss spectroscopy on the identification of plasmons: An example of graphene
  • 文献类型:   Article
  • 作  者:   LI JD, LIN ZJ, MIAO GY, ZHONG WL, XUE SW, LI Y, TAO ZY, WANG WH, GUO JD, ZHU XT
  • 作者关键词:   high resolution electron energy los, spectroscopy, twodimensional energymomentum mapping, dipole scattering theory, scattering geometric factor, acoustic plasmon, graphene
  • 出版物名称:   SURFACE SCIENCE
  • ISSN:   0039-6028 EI 1879-2758
  • 通讯作者地址:  
  • 被引频次:   2
  • DOI:   10.1016/j.susc.2022.122067 EA MAR 2022
  • 出版年:   2022

▎ 摘  要

High-resolution electron energy loss spectroscopy (HREELS) is one of the most powerful methods to detect the dispersion of plasmons. However, we find that in the HREELS measurement, the scattering geometric configu-ration will seriously affect the identification of plasmons. Here, taking graphene as an example, using the HREELS capable of two-dimensional energy-momentum mapping combined with the intensity distribution cal-culations, we visually display the intensity distribution of the scattering geometric factor. We demonstrate that the energy loss peaks from the scattering geometric effect may be misinterpreted as the features of an acoustic plasmon. In any HREELS measurement, it is necessary to evaluate the effect of the scattering geometry quan-titatively to identify the intrinsic surface excitations.