• 文献标题:   Graphene Near-Degenerate Four-Wave Mixing for Phase Characterization of Broadband Pulses in Ultrafast Microscopy
  • 文献类型:   Article
  • 作  者:   CIESIELSKI R, COMIN A, HANDLOSER M, DONKERS K, PIREDDA G, LOMBARDO A, FERRARI AC, HARTSCHUH A
  • 作者关键词:   graphene, fourwave mixing, pulse shaping femtosecond laser, microscopy, phase retrieval
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   Univ Munich
  • 被引频次:   10
  • DOI:   10.1021/acs.nanolett.5b00893
  • 出版年:   2015

▎ 摘  要

We investigate near-degenerate four-wave mixing in graphene using femtosecond laser pulse shaping microscopy. Intense near-degenerate four-wave mixing signals on either side of the exciting laser spectrum are controlled by amplitude and phase shaping. Quantitative signal modeling for the input pulse parameters shows a spectrally flat phase response of the near-degenerate four-wave mixing due to the linear dispersion of the massless Dirac Fermions in graphene. Exploiting these properties we demonstrate that graphene is uniquely suited for the intrafocus phase characterization and compression of broadband laser pulses, circumventing disadvantages of common methods utilizing second or third harmonic light.