• 文献标题:   Facile synthesis of 2D nitrogen-containing porous carbon nanosheets induced by graphene oxide for high-performance supercapacitors
  • 文献类型:   Article
  • 作  者:   ZHANG X, FAN QY, ZHAO YY, WANG M, MENG YL, XIAO YH, LEI XT, YANG J
  • 作者关键词:  
  • 出版物名称:   SUSTAINABLE ENERGY FUELS
  • ISSN:   2398-4902
  • 通讯作者地址:   Dalian Univ Technol
  • 被引频次:   2
  • DOI:   10.1039/c8se00242h
  • 出版年:   2018

▎ 摘  要

Two-dimensional (2D) nitrogen-containing porous carbon nanosheets are prepared in the presence of graphene oxide (GO) as a structure-directing agent by a simple yet facile hydrothermal method. It is found that GO can effectively tune the morphologies of the hydrothermal carbonaceous products, resulting in the unique 2D structures. The as-obtained 2D nitrogen-containing porous carbon nanosheets as electrodes for supercapacitors exhibit a high specific capacitance of 301.6 F g(-1) at a current density of 0.5 A g(-1) and superior rate capability with a capacitance retention of 70.5% at a high current density of 20 A g(-1). The 2D nitrogen-containing porous carbon nanosheet electrodes also exhibit good cycling performance, possessing a high capacitance retention of over 92.3% after 5000 charge-discharge cycles at a current density of 5 A g(-1). Such superior electrochemical performance of the 2D nitrogen-containing porous carbon nanosheets could be attributed to the high pseudocapacitive effect of the nitrogen-containing species and the peculiar structural characteristics featuring a short ion transport distance and abundant porous channels.