• 文献标题:   Bright Multicolored Photoluminescence of Hybrid Graphene/Silicon Optoelectronics
  • 文献类型:   Article
  • 作  者:   LIU K, ZHU ZH, LI XJ, ZHANG JF, YUAN XD, GUO CC, XU W, QIN SQ
  • 作者关键词:   graphene, silicon, frequencyupconverted photoluminescence, broadband, hot carrier multiplication, hot carrier scattering
  • 出版物名称:   ACS PHOTONICS
  • ISSN:   2330-4022
  • 通讯作者地址:   Natl Univ Def Technol
  • 被引频次:   7
  • DOI:   10.1021/acsphotonics.5b00051
  • 出版年:   2015

▎ 摘  要

Graphene does not possess a band gap, and hot carrier relaxation in graphene is an ultrafast processs. This leads to a very low emission efficiency of graphene. We demonstrate bright multicolored frequency-upconverted photoluminescence from graphene via three-photon absorption by femtosecond laser injection at a communication wavelength 1.57 mu m. The broadband and multiwavelength emission from graphene is based on the model of ultrafast electron-hole pair recombination and asymmetrical energized electron-hole radiation recombination in graphene. Furthermore, we show photoluminescence variation with blue light emission in the graphene/silicon hybrid system, with 2-3 orders of emission efficiency increase. The results demonstrate hot carrier multiplication and hot carrier scattering in graphene and could help to study the population inversion and broadband lasing of graphene.