• 文献标题:   Catalytic activities enhanced by abundant structural defects and balanced N distribution of N-doped graphene in oxygen reduction reaction
  • 文献类型:   Article
  • 作  者:   BAI XG, SHI YT, GUO JH, GAO LG, WANG K, DU Y, MA TL
  • 作者关键词:   ndoping graphene, oxygen reduction reaction, ndistribution, structural defect
  • 出版物名称:   JOURNAL OF POWER SOURCES
  • ISSN:   0378-7753 EI 1873-2755
  • 通讯作者地址:   Dalian Univ Technol
  • 被引频次:   34
  • DOI:   10.1016/j.jpowsour.2015.10.081
  • 出版年:   2016

▎ 摘  要

N-doped graphene (NG) is a promising candidate for oxygen reduction reaction (ORR) in the cathode of fuel cells. However, the catalytic activity of NG is lower than that of commercial Pt/C in alkaline and acidic media. In this study, NG samples were obtained using urea as N source. The structural defects and N distribution in the samples were adjusted by regulating the pyrolysis temperature. The new NG type exhibited remarkable catalytic activities for ORR in both alkaline and acidic media. (C) 2015 Elsevier B.V. All rights reserved.