• 文献标题:   Controlling Graphene Ultrafast Hot Carrier Response from Metal-like to Semiconductor-like by Electrostatic Gating
  • 文献类型:   Article
  • 作  者:   SHI SF, TANG TT, ZENG B, JU L, ZHOU Q, ZETTL A, WANG F
  • 作者关键词:   graphene, terahertz, hot carrier, pumpprobe
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   Univ Calif Berkeley
  • 被引频次:   78
  • DOI:   10.1021/nl404826r
  • 出版年:   2014

▎ 摘  要

We investigate the ultrafast terahertz response of electrostatically gated graphene upon optical excitation. We observe that the photoinduced terahertz absorption increases in charge neutral graphene but decreases in highly doped graphene. We show that this transition from semiconductor-like to metal-like response is unique for zero bandgap materials such as graphene. In charge neutral graphene photoexcited hot carriers effectively increase electron and hole densities and increase the conductivity. In highly doped graphene, however, photoexcitation does not change net conducting carrier concentration. Instead, it mainly increases electron scattering rate and reduce the conductivity.